Abstract

A systematic characterization of Co-doped BaFe2As2(Ba-122) thin films has been carried out. Two samples were available, one grown on CaF2substrate and the other on MgO with an Fe buffer layer. The goal was to investigate films’ magnetic and superconducting properties, their reciprocal interplay, and the role played by the Fe buffer layer in modifying them. Morphological characterization and Energy Dispersive X-ray analyses on the Fe-buffered sample demonstrate the presence of diffused Fe close to the Co-doped Ba-122 outer surface as well as irregular holes in the overlying superconducting film. These results account for hysteresis loops obtained with magneto-optic Kerr effect measurements and observed at both room and low temperatures. The magnetic pattern was visualized by magneto-optical imaging with an indicator film. Moreover, we investigated the onset of superconductivity through a measure of the superconducting energy gap. The latter is strictly related to the decay time of the excitation produced by an ultrashort laser pulse and has been determined in a pump-probe transient reflectivity experiment. A comparison of results relative to Co-doped Ba-122 thin films with and without Fe buffer layer is finally reported.

Highlights

  • Tremendous efforts have been made to obtain reliable information on fundamental properties of iron-based superconductors (IBS), such as superconducting energy gaps, nature of excitation assisting Cooper pair formation, andmagnetism

  • Many applications based on Josephson effect have been proposed and realized, for example, Superconducting Quantum Interference Devices (SQUIDs) [1] and Single Flux Quantum (SFQ) devices

  • We report on additional characterization of Codoped Ba-122 samples with magneto-optical imaging (MOI) and magneto-optical Kerr effect (MOKE)

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Summary

Introduction

Tremendous efforts have been made to obtain reliable information on fundamental properties of iron-based superconductors (IBS), such as superconducting energy gaps, nature of excitation assisting Cooper pair formation, and (ferro)magnetism. In IBS, ultrafast spectroscopy has been used to reveal the existence of pseudogap states [8], competition between SDWs and superconducting states [13] and to understand the role of interband interactions and gap symmetry [14]. This technique ultrafast spectroscopy has been used to investigate quasiparticle (QP) dynamics in Ba-122 family, proving its ability to reveal the multigap nature of such superconductors [15]. By means of different optical techniques, namely, MOKE, MOI, and ultrafast spectroscopy, we could establish the role of Fe buffer layers on magnetic and superconducting properties of our Ba-122 samples

Materials and Experimental Set-Up
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