Abstract

We grew pure 1T/2H-TaS2 single crystals via the chemical vapor transport (CVT) method and introduced defects into the samples by quenching. We systematically investigated the influence of defects on charge–density–wave (CDW) and superconductivity (SC) in 1T and 2H-TaS2. The defects can induce SC to 1T-TaS2 system, and inhibit the commensurate CDW (CCDW) and Mott insulator phase, the superconducting transition temperature (TcOnset) is about 2.5K and the zero resistivity temperature (Tczero) is about 0.7K. For 2H-TaS2, the defects nearly have no effect on CDW, while TcOnset is increased to about 2.7K. The magnetization hysteresis loops show typical type-II superconductor behaviors for both 1T and 2H-TaS2 systems.

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