Abstract

AbstractMethylation of the phenylhydrazone derived from 8‐oxo‐8H‐indeno[1,2‐d]‐1,2,3‐thiadiazole 5 with Meerwein's reagent furnishes the two methylated products 7 and 8. Single crystal X‐ray analyses of these compounds reveal no significant S…NPh interaction, thus excluding a thiapentalene structure.

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