Abstract

Employment of the non-trivial proximity effect in superconductor/ferromagnet (S/F) heterostructures for the creation of novel superconducting devices requires accurate control of magnetic states in complex thin-film multilayers. In this work, we study experimentally in-plane transport properties of microstructured Nb/Co multilayers. We apply various transport characterization techniques, including magnetoresistance, Hall effect, and the first-order-reversal-curves (FORC) analysis. We demonstrate how FORC can be used for detailed in situ characterization of magnetic states. It reveals that upon reduction of the external field, the magnetization in ferromagnetic layers first rotates in a coherent scissor-like manner, then switches abruptly into the antiparallel state and after that splits into the polydomain state, which gradually turns into the opposite parallel state. The polydomain state is manifested by a profound enhancement of resistance caused by a flux-flow phenomenon, triggered by domain stray fields. The scissor state represents the noncollinear magnetic state in which the unconventional odd-frequency spin-triplet order parameter should appear. The non-hysteretic nature of this state allows for reversible tuning of the magnetic orientation. Thus, we identify the range of parameters and the procedure for in situ control of devices based on S/F heterostructures.

Highlights

  • Competition between spin-polarized ferromagnetism and spinsinglet superconductivity leads to a variety of interesting phenomena including the possible generation of the odd-frequency spin-triplet order parameter [1,2,3]

  • Even a long-range supercurrent cannot be automatically ascribed to the triplet order. (ii) The supercurrent strongly depends on a usually unknown domain structure in F [23,30,36] and flux quantization in S [37,38], both influenced by size and geometry. (iii) The long-range spin-triplet supercurrent appears only in the noncollinear magnetic state [5,9,10,11,12]

  • Resistances are measured with Iac = 10 μA for S1 and 20 μA for S2, which correspond to approximately equal small current densities in both MLs. Both MLs show a double transition, which could be attributed to different critical temperatures in S and S′ layers, T′c(S′) < Tc(S)

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Summary

Introduction

Competition between spin-polarized ferromagnetism and spinsinglet superconductivity leads to a variety of interesting phenomena including the possible generation of the odd-frequency spin-triplet order parameter [1,2,3] In recent years, this exotic state has been extensively studied both theoretically [4,5,6,7,8,9,10,11,12,13,14,15,16,17] and experimentally [18,19,20,21,22,23,24,25,26,27,28,29,30,31,32,33,34,35] in various superconductor/ferromagnet (S/F) heterostructures. The need for establishing experimental characterization techniques for the in situ monitoring of magnetic states in S/F micro- and nanoscale devices is our main motivation

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