Abstract
Using first-principles calculations, we investigated the impact of chromium (Cr) and vanadium (V) impurities on the magnetic anisotropy and spin polarization in Fe/MgO magnetic tunnel junctions. It is demonstrated, using layer resolved anisotropy calculation technique, that while the impurity near the interface has a drastic effect in decreasing the perpendicular magnetic anisotropy (PMA), its position within the bulk allows maintaining high interfacial PMA while reducing the bulk magnetization and correlatively the easy-plane demagnetizing energy. As a result, the effective magnetic anisotropy tends to increase as a function of the Cr or V concentration resulting in an increase in the critical magnetic thickness at which the crossover from out-of-plane to in-plane anisotropy takes place. At the same time, the interfacial spin polarization is not affected by the magnetic layer bulk doping by Cr or V impurities and even enhanced in most situations thus favoring an increase of tunnel magnetoresistance (TMR) amplitude.
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