Abstract

Ti substituting Ru in Sr$_2$RuO$_4$ in small concentrations induces incommensurate spin density wave order with a wave vector $\boldsymbol{Q} \simeq (2 \pi /3, 2 \pi /3)$ corresponding to the nesting vector of two out of three Fermi surface sheets. We consider a microscopic model for these two bands and analyze the correlation effects leading to magnetic order through non-magnetic Ti-doping. For this purpose we use a position dependent mean field approximation for the microscopic model and a phenomenological Ginzburg-Landau approach, which both deliver consistent results and allow us to examine the inhomogeneous magnetic order. Spin-orbit coupling additionally leads to spin currents around each impurity, which in combination with the magnetic polarization produce a charge current pattern. This is also discussed within a gauge field theory in both charge and spin channel. This spin-orbit coupling effect causes an interesting modification of the magnetic structure, if currents run through the system. Our findings allow a more detailed analysis of the experimental data for Sr$_{2}$Ru$_{1-x}$Ti$_{x}$O$_{4}$. In particular, we find that the available measurements are consistent with our theoretical predictions.

Highlights

  • Motivated by the discovery of unconventional superconductivity, Sr2RuO4 has been studied extensively for well over two decades due to its many intriguing properties [1,2,3,4]

  • Incommensurate (IC) correlations have been experimentally observed at the wave vector Q (2π /3, 2π /3) [10,11,12,13,14,15,16], very consistent with theoretical predictions [17,18,19,20,21]

  • We find that the dominant magnetic correlation in the pure system is connected with the four IC wave vectors Q (±2π /3, 0) and (0, ±2π /3), which, if strong enough, would lead to a spin density wave state based on these wave vectors

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Summary

INTRODUCTION

Motivated by the discovery of unconventional superconductivity, Sr2RuO4 has been studied extensively for well over two decades due to its many intriguing properties [1,2,3,4]. Due to its strongly correlated Fermi-liquid properties in the normal state Sr2RuO4 with its single-layer perovskite structure has been considered a two-dimensional analog of 3He [8,9]. Sr2RuO4 falls barely short of establishing magnetic longrange order originating from the strong IC correlations It was, found that replacing some Ru4+ by nonmagnetic Ti4+ (3d0) induces magnetic order already at rather low Ti concentrations, x > 0.025 in Sr2Ru1−xTixO4 [25]. From the microscopic model of the α-β bands including spin-orbit coupling we develop a mean-field theory for a spatially dependent magnetization of the two involved 4d orbitals and determine the pattern of magnetic order around a single impurity. We will analyze the magnetic structure induced by nonmagnetic impurities based on a microscopic model of the α-β bands including the effects of spin-orbit coupling (Sec. II). These phenomena may allow for interesting probes of the magnetic properties of such a system

The model Hamiltonian
Self-consistent T -matrix approximation
Local mean-field approximation
PHENOMENOLOGICAL APPROACH FOR A SYSTEM WITH MANY IMPURITIES
Ginzburg-Landau theory
Magnetic order with several impurities
EFFECTIVE FIELD THEORY
Formulation and basic results
Correlation functions connecting gauge fields and potentials
Impurity-induced spin currents
Charge currents induced by magnetization pattern
Spin polarization induced by external charge currents
CONCLUSION
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