Abstract
Honey is a high-value product that proscribes adulteration. Authentication of pure honey is an imperative act that can disregard the adverse impacts brought by fraudsters on honey producers and consumers. A reliable method that can detect food adulteration that is nondestructive, rapid, and efficient can help maintain product authenticity. This study investigated the potential of a near-infrared hyperspectral imaging (NIR-HSI) system combined with supervised classification techniques for the classification of honey samples from different botanical origins that were adulterated with sugar cane syrup at 20 % and 40 % w/w. Reflectance and transflectance modes of measurement were used to obtain honey spectral images from 864.53 nm to 1700 nm. Supervised classification algorithms, namely, stepwise discriminant analysis (SDA), support vector machine (SVM), and k-nearest neighbors (kNN) were used for the classification based on whole spectral data and feature selected spectral data. The best classification model from reflectance mode was observed from SDA based on a leave-one-out cross-validation (LOOCV) method with a test accuracy of 95 %. For transflectance mode, the classification model developed from SDA based on a LOOCV method provided better test set accuracy of 100 %. The classification performance levels of the models developed from SVM and kNN were lower with the use of the whole wavelength region. Moreover, the classification performance levels of SVM and kNN using the selected features by the SDA greatly increased, however, they were not as good as from using SDA alone. The classifier maps created using SDA and predicting the averaged spectra of all pixels in the image with 10-discriminant functions for each mode of measurement displayed a two-dimensional image that had a distinct colour pertaining to a particular class that could easily discriminate one class from another.
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