Abstract
Traffic is a significant pollution source in cities and has caused various health and environmental concerns worldwide. Therefore, the improved understanding of traffic impacts on particle concentrations could help mitigate air pollution. In this study, field measurements were conducted beside an arterial road in Shanghai, China, to obtain the fine-scale temporal variations in traffic volumes, meteorological parameters, and size-resolved particle concentrations. The generalized additive model was developed to reveal their associations under different analysis intervals (time scales). Results indicate that on-road traffic greatly increased the concentration and variability of roadside particles. Variations of roadside fine particles (<1 μm, having high homogeneity) closely followed those at the background point, but background variations of coarse particles (having high heterogeneity) were negligible compared with the roadside point. Roadside particles showed high variability on the 10-s scale and presented frequent stochastic spikes above the background level. The particle variability was greatly reduced on the 60-min scale, exhibiting stable variations. The association between traffic and roadside particle variations was weak on a fine temporal scale (5-min scale). However, the association showed a pronounced increase when the analysis interval was increased (60-min scale). This is because extending the analysis interval could reduce the influence of random factors (sample randomness) and emission lagging effects on the results. Moreover, with the increase of the analysis interval, the improvement of associations between variables can be well characterized by exponential curves, which could help determine the optimal analysis interval. Additionally, heavy-duty vehicles showed a lot more significant influence on particle variations compared with that of light-duty vehicles, and should be regarded as the key governance target for on-road pollution control. These findings broaden the knowledge of traffic impacts on particle concentrations, which could provide implications in air pollution abatement.
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