Impact of intensity variability of the Asian summer monsoon anticyclone on the chemical distribution in the upper troposphere and lower stratosphere

Abstract

During the Asian summer monsoon (ASM) season, the process of stratosphere–troposphere exchange significantly affects the concentration and spatial distribution of chemical constituents in the upper troposphere and lower stratosphere (UTLS). However, the effect of the intensity of the Asian summer monsoon anticyclone (ASMA) on the horizontal distribution of chemical species within and around the ASMA, especially on the daily time scale, remains unclear. Here, the authors use the MERRA-2 reanalysis dataset and Aura Microwave Limb Sounder observations to study the impact of ASMA intensity on chemical distributions at 100 hPa during the ASM season. The intraseasonal variation of ASMA is classified into a strong period (SP) and weak period (WP), which refer to the periods when the intensity of ASMA remains strong and weak, respectively. The relatively low ozone (O3) region is found to be larger at 100 hPa during SPs, while its mixing ratio is lower than during WPs in summer. In June, analysis shows that the O3 horizontal distribution is mainly related to the intensity of AMSA, especially during SPs in June, while deep convections also impact the O3 horizontal distribution in July and August. These results indicate that the intraseasonal variation of the ASMA intensity coupled to deep convection can significantly affect the chemical distribution in the UTLS region during the ASM season.摘要亚洲夏季风期, 平流层–对流层物质交换过程能显著影响上对流层下平流层化学成分的浓度变化和空间分布. 然而, 亚洲夏季风反气旋强度的季节内变化对其内部和周围地区化学成分水平分布的影响尚不清楚. 本文将亚洲夏季风反气旋划分为季节内强周期和弱周期, 发现当亚洲夏季风反气旋更强时, 100 hPa O3低值区的面积更大, O3浓度更低. 但是这种影响主要体现在6月份, 7, 8月的O3水平分布还受东南亚地区深对流的影响. 这些结果表明亚洲夏季风反气旋强度和深对流的季节内变化可以显著影响亚洲夏季风期上对流层下平流层的化学分布.