Abstract

Soils are key to ecosystems and human societies, and their critical importance requires a better understanding of how they evolve through time. However, identifying the role of natural climate change versus human activity (e.g. agriculture) on soil evolution is difficult. Here we show that for most of the past 12,300 years soil erosion and development were impacted differently by natural climate variability, as recorded by sediments deposited in Lake Dojran (Macedonia/Greece): short-lived ( < 1,000 years) climatic shifts had no effect on soil development but impacted soil erosion. This decoupling disappeared between 3,500 and 3,100 years ago, when the sedimentary record suggests an unprecedented erosion event associated with the development of agriculture in the region. Our results show unambiguously how differently soils evolved under natural climate variability (between 12,300 and 3,500 years ago) and later in response to intensifying human impact. The transition from natural to anthropogenic landscape started just before, or at, the onset of the Greek ‘Dark Ages’ (~3,200 cal yr BP). This could represent the earliest recorded sign of a negative feedback between civilization and environmental impact, where the development of agriculture impacted soil resources, which in turn resulted in a slowdown of civilization expansion.

Highlights

  • Soil systems are key components of a broad range of ecosystems

  • We investigated the relative impact of climate variability and human activity on soil systems during the Late Glacial and Holocene in south-eastern Europe

  • Lithium isotopes (7Li and 6Li) fractionate during clay formation, whereby 6Li is preferentially enriched in clay minerals compared to 7Li17,18

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Summary

Introduction

Soil systems are key components of a broad range of ecosystems. Their development via chemical weathering and mineral dissolution consumes carbon dioxide, and plays a substantial role in regulating the carbon cycle and Earth’s climate[1,2,3]. We used uranium and lithium isotopes in lacustrine sedimentary deposits as proxies for soil erosion and development, respectively. In weathering profiles where primary minerals are continuously weathered into clays, soils are increasingly enriched in 6Li, preferentially retained in clays over 7Li. decreasing δ7Li values reflect increasing clay formation, used as a proxy for the extent of soil development (Supplementary Fig. S7)[20].

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