Impact of changes in refractive indices of secondary organic aerosols on precipitation over China during 1980–2019

Abstract

Secondary organic aerosols (SOAs), which include both colorless and colored carbonaceous aerosols, represent a major type of aerosol globally. Previous studies have reported that colored aerosols drive the well-known precipitation changes over southern China called the south-flood north-drought (SFND). Considering the highest concentration of SOA in China, SOAs can cause fluctuations in the precipitation system over China. However, studies on the climatic effects of SOAs over East Asia are scarce owing to the chemical complexity of SOAs and high computational cost. Therefore, to investigate the effect of SOAs on the precipitation change over China, we implemented an SOA scheme using empirical parameters in the chemistry-climate model. We performed a control and two sensitivity simulations depending on the difference in refractive indices of SOAs to elucidate the effects of light absorption by SOAs on precipitation. Our results suggest that strong light absorption by SOAs strengthens the convective precipitation over southern China following the enhancement of atmospheric stability with a secondary circulation effect. However, the surface temperature changes caused by SOAs shift the jet core if weak light absorption by SOAs is assumed, causing a strong downdraft in the mid-troposphere and decreasing humidity over south-eastern China. Therefore, precipitation was significantly reduced over southern China. Our results show that light-absorbing SOAs have had a significant impact on precipitation in southern China for the past few decades. Furthermore, the apparent difference in mechanisms of precipitation change between strong and weak light absorption by SOAs suggests the importance of choosing suitable refractive indices for SOAs in the climate–atmospheric chemistry model.