Impact of atmospheric circulation patterns on properties and regional transport pathways of aerosols over Central-West Asia: Emphasizing the Tibetan Plateau

Abstract

The Tibetan Plateau (TP), as a remote and sparsely populated area, is regularly exposed to polluted air masses sourcing from surrounding regions. Atmospheric circulation, as the major driving force generating long-range transport processes of air pollutants, contributes to high-pollution episodes on the TP. Therefore, using reanalysis data from the European Centre for Medium-Range Weather Forecasts for the 2000–2019 period, this paper first classified atmospheric circulation patterns over the study area into nine types (type 1 – type 9). Among them, circulation types 1, 2, 6, and 8 mainly occurred in spring and winter, while circulation types 3, 4, 5, 7, and 9 primarily occurred in summer and autumn. Second, ground-based and satellite remote sensing data were combined to investigate the impact of atmospheric circulation patterns on the properties of aerosols over Central-West Asia and their surrounding areas. We detailed how the atmospheric circulation patterns impacted the aerosol optical depth, Ångström exponent, and aerosol types at different Aerosol Robotic Network sites in the study area. The results obtained from ground-based data were further verified by those from satellite remote sensing data. Third, backward trajectories and the corresponding potential source contribution function based on the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model were used to explore the impact of atmospheric circulation patterns on regional transport pathways of aerosols. It was found that under circulation types 1, 2, 6, and 8, few HYSPLIT trajectories were sourced from the south direction, while under circulation types 3, 4, 5, 7, and 9, the trajectories originating from the south increased significantly, which could be attributed to the summer monsoon.