Abstract

Powders and their mixtures are elemental for many industries (e.g., food, pharmaceutical, mining, agricultural, and chemical). The properties of the manufactured products are often directly linked to the particle properties (e.g., particle size and shape distribution) of the utilized powder mixtures. The most straightforward approach to acquire information concerning these particle properties is image capturing. However, the analysis of the resulting images often requires manual labor and is therefore time-consuming and costly. Therefore, the work at hand evaluates the suitability of Mask R-CNN—one of the best-known deep learning architectures for object detection—for the fully automated image-based analysis of particle mixtures, by comparing it to a conventional, i.e., not machine learning-based, image analysis method, as well as the results of a trifold manual analysis. To avoid the need of a laborious manual annotation, the training data required by Mask R-CNN are produced via image synthesis. As an example for an industrially relevant particle mixture, endoscopic images from a fluid catalytic cracking reactor are used as a test case for the evaluation of the tested methods. According to the results of the evaluation, Mask R-CNN is a well-suited method for the fully automatic image-based analysis of particle mixtures. It allows for the detection and classification of particles with an accuracy of 42.7% for the utilized data, as well as the characterization of the particle shape. Also, it enables the measurement of the mixture component particle size distributions with errors (relative to the manual reference) as low as −2±5 for the geometric mean diameter and −6±5% for the geometric standard deviation of the dark particle class of the utilized data, as well as −8±4% for the geometric mean diameter and −6±2% for the geometric standard deviation of the light particle class of the utilized data. Source code, as well as training, validation, and test data publicly available.

Highlights

  • Powders are crucial for many branches of modern industry

  • The initially light particles become darker and less catalytically active over time, so that fresh and light particles have to beintroduced to the reactor. This results in a particle mixture featuring two classes: dark and light particles

  • To avoid the laborious creation of the training data via manual annotation, we propose the use of image synthesis

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Summary

Introduction

Powders are crucial for many branches of modern industry. A prominent example is the chemical industry, where approximately 60 % of the products are powders themselves and another 20 % require powders during their production (in Europe) [1]. A prominent example for the relevance of particle mixtures in the chemical industry is fluid catalytic cracking (FCC), which is considered to be the most important conversion method from the realm of petrochemistry [3]. FCC reactors are filled with catalyst particles, which are progressively loaded with coke during the continuous cracking process. The initially light particles become darker and less catalytically active over time, so that fresh (or regenerated) and light particles have to be (re)introduced to the reactor. This results in a particle mixture featuring two classes: dark and light particles

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