Abstract
The v′=0–4 levels of the 3dπ 1Δg state and v′=0–3 levels of the 3dπ 3Δ2g state of O2 have been identified and studied by multiphoton ionization and polarization techniques. The observed levels exhibit no detectable perturbation except for rather large Λ doubling probably due to L uncoupling, and heterogeneous predissociation probably by a Πg valence state. The observation of large amounts of O+ for the higher vibrational levels suggests large non-Franck–Condon effects in the ionization process.
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