Abstract
Stimulus-responsive actuators play a vital role in the new generation of intelligent systems. However, poor mechanical performance, complicated fabrication processes, and the inability to complex deformation limit their practical applications. Herein, these challenges are overcome via designing a strong hygrothermic wood actuator with asymmetric water affinity. The actuator is readily constructed by sandwiching polypyrrole-coated wood with a Ni complex hygroscopic gel top layer for moisture absorption and a polyimide bottom layer as the water barrier. The resulting hygrothermic wood spontaneously stretches and bends itself in response to moisture and thermal/light stimulation. A robotic hand and a series of grippers made of hygrothermic wood demonstrate dexterous object-hand interactions during grasping and holding, while the reversible hygrothermic property allows the actuator to be potentially applied in fire rescue scenarios to rescue trapped objects. A combination of good mechanical properties, multi-stimulus-response, complex deformation, wide working temperature range, low manufacturing cost, and biocompatibility are simultaneously realized by one device. It is thus believed that such a strong wood actuator will open up a new avenue for building intelligent robotic hand systems.
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