Hydrodynamics and Mass Transfer in an Airlift Loop Reactor: Comparison between Using Two Kinds of Spargers

Abstract

The effects of different spargers on the hydrodynamics and mass transfer of an airlift loop reactor were investigated. The gas holdup, liquid loop velocity, and volumetric mass transfer coefficient of the reactor were tested using a ring orifice distributor and a jet nozzle. The study was conducted in a 6 m high airlift loop reactor at a superficial gas velocity of 0.01~0.04 m/s, and the superficial liquid velocity was maintained at 0.0154 m/s. The results showed that using the jet nozzle provided a higher gas holdup, liquid loop velocity, and mass transfer. When the superficial gas velocity was less than 0.0325 m/s, the liquid loop velocity generated by the jet nozzle was approximately 1.1-fold higher than that generated by the ring orifice distributor, and the disparity in gas holdup between the riser and downcomer enhanced the power of liquid circulation. When the superficial gas velocity was more than 0.0325 m/s, the jet kinetic power dominated the improvement in the liquid loop velocity, and the energy input from the nozzle to the airlift loop reactor was greater than 10.8 J/(s·m2). This indicated a threshold of energy input for overcoming the friction loss. In this situation, the liquid loop velocity in the jet form increased considerably, thus favoring the mixing performance and temperature uniformity of the reactor. It was also of significance for avoiding the formation of a flow dead zone in scale-up airlift loop reactors.