Abstract

The detection of unusual 'mirage' energy bands in photoemission spectra of single-atom layers of iron selenide reveals the probable cause of high-temperature superconductivity in these artificial structures. See Letter p.245 Bulk iron selenide (FeSe) is a superconductor with a critical temperature Tc = 8 K, but superconductivity is substantially enhanced in single-unit cell films of FeSe grown on strontium titanate (SrTiO3 or STO) substrates, where superconducting energy gaps open at temperatures close to the boiling point of liquid nitrogen (77 K). This raises the question of whether the substrate has a contributory role in this enhancement. Zhi-Xun Shen and colleagues report high-resolution angle-resolved photoemission spectroscopy (ARPES) results that reveal bosonic modes (thought to be oxygen optical phonons) in the SrTiO3 substrate coupling to electrons in the FeSe overlayer to facilitate high-temperature superconductivity. Such coupling helps superconductivity in most channels, so the pairing enhancement described here may well work for other superconducting materials, as well as for FeSe.

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