Abstract
Despite significant interest in persistent luminescence materials, the focus of all recent works remains on the exploitation of materials in powder form. Here, a new point of view based on persistent luminescence in single crystals is presented. The garnet crystals [(Gd0.67Y0.33)3-xCex)](Al2-yCry)Ga3O12 and [(Gd0.33Y0.67)3-xCex](Al2-yCry)Ga3O12 (GYAGG) codoped with Ce3+ and different concentrations of Cr3+ have been elaborated and their persistent luminescence properties are fully characterized within this work. The persistent luminescence of Ce3+, Cr3+-codoped GYAGG single crystals is optimized due to their high optical quality, very good crystallinity and a volume effect where the whole material can be excited and charged by the excitation light. Furthermore, thanks to their transparency, robustness and homogeneity; in-depth optical spectroscopy characterization is possible, shedding light on the mechanism responsible for the afterglow.
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