Abstract

Three-dimensional topological insulators (TIs) in proximity with superconductors are expected to exhibit exotic phenomena, such as topological superconductivity (TSC) and Majorana-bound states (MBS), which may have applications in topological quantum computation. In superconductor–TI–superconductor Josephson junctions, the supercurrent versus the phase difference between the superconductors, referred to as the current–phase relation (CPR), reveals important information including the nature of the superconducting transport. Here, we study the induced superconductivity in gate-tunable Josephson junctions (JJs) made from topological insulator BiSbTeSe2 with superconducting Nb electrodes. We observe highly skewed (non-sinusoidal) CPR in these junctions. The critical current, or the magnitude of the CPR, increases with decreasing temperature down to the lowest accessible temperature (T ~ 20 mK), revealing the existence of low-energy modes in our junctions. The gate dependence shows that close to the Dirac point the CPR becomes less skewed, indicating the transport is more diffusive, most likely due to the presence of electron/hole puddles and charge inhomogeneity. Our experiments provide strong evidence that superconductivity is induced in the highly ballistic topological surface states (TSS) in our gate-tunable TI-based JJs. Furthermore, the measured CPR is in good agreement with the prediction of a model which calculates the phase-dependent eigenstate energies in our system, considering the finite width of the electrodes, as well as the TSS wave functions extending over the entire circumference of the TI.

Highlights

  • Three-dimensional (3D) topological insulators (TIs) are a new class of quantum matters and are characterized by an insulating bulk and conducting topological surface states (TSS)

  • Our BiSbTeSe2 crystals are among the most bulk-insulating 3D TIs, where the Fermi energy lies within the bulk bandgap and inside the TSS, as verified by the angle-resolved photoemission spectroscopy (ARPES) and transport measurements.[29]

  • We have recently observed an anomalous enhancement of the critical current in Josephson junctions (JJs) based on BiSbTeSe2 nanoribbons, demonstrating the induced superconductivity in the TSS.[28]

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Summary

Introduction

Three-dimensional (3D) topological insulators (TIs) are a new class of quantum matters and are characterized by an insulating bulk and conducting topological surface states (TSS). Our BiSbTeSe2 crystals are among the most bulk-insulating 3D TIs, where the Fermi energy lies within the bulk bandgap and inside the TSS, as verified by the angle-resolved photoemission spectroscopy (ARPES) and transport measurements.[29] Exfoliated thin films of this material exhibit ambipolar field effect, as well as several signatures of topological transport through the spin-helical Dirac fermion TSS, including the half-integer quantum Hall effect and π Berry phase.[29,30] we have recently observed an anomalous enhancement of the critical current in JJs based on BiSbTeSe2 nanoribbons, demonstrating the induced superconductivity in the TSS.[28] Figure 1a shows a scanning electron microscope (SEM) image of an asymmetric SQUID with a BiSbTeSe2 flake (sample A).

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