Abstract
HighlightsFacile fabrication of high-transconductance (>10 mS) and highly elastic all-polymer organic electrochemical transistors was presented using gelatin-based electrolyte supporting printed PEDOT:PSS/LiTFSI microstructures.PEDOT:PSS/LiTFSI wrinkled microelectrodes and imprinted 3D-microstructured channel/electrolyte interface allowed biaxial stretchability of 100% strain and performance preservation after 1000 cycles of 80% strain.The glycerol-soaked elastic gelatin electrolyte also permitted long-term environmental stability for months and enabled readily recyclable device, paving the way to wide applications spanning from artificial synapses to wearable sensing.
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