Abstract
The reaction of Fe-atoms with CO2 was studied in the temperature range of 1330 K ⩽ T ⩽ 2650 K at pressures between 1.0 and 1.6 bar in a shock wave reactor. Resonance absorption spectroscopy was applied for time-resolved measurement of Fe-atoms, O-atoms, and CO-molecules in initial gas mixtures containing Fe(CO)5 and CO2, highly diluted in argon. The experiments showed at early reaction time an Fe-consumption and a simultaneous CO formation which was interpreted by reaction R2 (explained below):
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