Abstract

Analysis of the structure of magnetooptic resonances of second order in laser radiation intensity, caused by resonance Raman scattering of radiation by the Zeeman sublevels split by the magnetic field and by saturation effects, has been until recently the basic content of nonlinear Zeeman spectroscopy. The present study is devoted to theoretical and experimental investigations of higher order nonlinear magnetooptic resonances. Rules are established, relating the various quantum-mechanical characteristics of atoms and molecules with high-order parameters of magnetooptic resonances. It is shown that these resonances make it possible to obtain information on relaxation of high rank multipole moments of electron shells.

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