Abstract

The use of indium–gallium–zinc oxide (IGZO) has paved the way for high-resolution uniform displays or integrated circuits with transparent and flexible devices. However, achieving highly reliable devices that use IGZO for low-temperature processes remains a technological challenge. We propose the use of IGZO thin-film transistors (TFTs) with an ionic-liquid gate dielectric in order to achieve high-density carrier-accumulated IGZO TFTs with high reliability, and we discuss a distinctive mechanism for the degradation of this organic–inorganic hybrid device under long-term electrical stress. Our results demonstrated that an ionic liquid or gel gate dielectric provides highly reliable and low-voltage operation with IGZO TFTs. Furthermore, high-density carrier accumulation helps improve the TFT characteristics and reliability, and it is highly relevant to the electronic phase control of oxide materials and the degradation mechanism for organic–inorganic hybrid devices.

Highlights

  • (a) Image and schematic cross-sectional view of the indium–gallium–zinc oxide (IGZO) thin-film transistors (TFTs) with ionic liquid

  • We present the application of IGZO TFTs with an ionic-liquid gate dielectric in order to achieve high reliability, and we discuss a mechanism for the device degradation of this organic–inorganic hybrid device under long-term electrical stress

  • Lee et al confirmed that the IGZO TFT degradation follows this relation[22]

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Summary

Introduction

(a) Image and schematic cross-sectional view of the IGZO TFT with ionic liquid. The underside image is the cross-sectional cut between points A and B, which are shown in the upper TFT image. (b) EMIM-TFSI ionic liquid structure. (c) Transfer characteristics and hysteresis curve of the IGZO TFTs with ionic liquid and SiO2 gate insulators. (d) Fifty-cycle measurement of the IGZO TFTs with ionic-liquid gate dielectric and gate leakage current, where the maximum values of Vgs are 2 and 20 V for the ionic-liquid and thermal SiO2 gate insulator TFTs, respectively, and Vds is 0.1 V. For low-voltage operation, insulating materials that can accumulate carriers at a high density in a semiconductor film are necessary. Some studies have demonstrated low-voltage-operation IGZO TFTs with high-capacitance and high-k material gate insulators for driving OLED devices[9,10,11]. The reliability under long-term electrical stress in an organic–inorganic combination has not been discussed. Determining the electrical stress reliability of IGZO TFTs by using an ionic-liquid gate dielectric has important implications for the application of organic–inorganic hybrid devices. We present the application of IGZO TFTs with an ionic-liquid gate dielectric in order to achieve high reliability, and we discuss a mechanism for the device degradation of this organic–inorganic hybrid device under long-term electrical stress

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