Abstract

Here we report the direct measurement of the nonlinear refractive index coefficient of liquids by using the Z-scan method with broadband pulsed THz beam. The results fit with conventional Z-scan analytics well. We estimate the nonlinear refractive index coefficient n <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</sub> of liquids through the use of the theoretical treatment that takes the ionic vibrational contribution into account. This estimation correlates with experimental data obtained.

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