Abstract
High CO2 separation performance on a microporous MOF incorporting nano-cages and an ultra-high density of dual-side open metal sites is reported.
Highlights
Developing efficient adsorbents for CO2 separation is the crucial step of CO2 sequestration. which has found many applications, including in carbon capture from flue gas and natural gas purification
Many adsorbents have been reported in the past few decades, developing efficient adsorbents with high separation selectivity and excellent capacity is technically challenging due to the trade-off effect between the adsorption capacity and selectivity
The preferential adsorption of alkenes to alkanes could be attributed to the p-electrons of alkenes, which could give back donations to open metal sites of Metal– organic frameworks (MOFs)
Summary
Developing efficient adsorbents for CO2 separation is the crucial step of CO2 sequestration. which has found many applications, including in carbon capture from flue gas and natural gas purification. This work reports the CO2 separation performance of a microporous MOF, which comprises nano-cages and an ultra-high density of dualside open metal sites. The outstanding separation performance can be attributed to the combined effects of nano-cages and the high density of open metal sites.
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