Abstract
A family of heterometallic NbU-3-Mn/MIII compounds were synthesized through postsynthetic exchange of MIII ions of a pentanuclear MnII-based metal-organic framework (NbU-3-Mn, where NbU denotes Ningbo University) for enhancing the gas-separation performance. Significantly, NbU-3-Mn/Fe has a C2H2/CO2 separation selectivity similar to that of NbU-3-Mn but exhibits enhanced dynamic separation of C2H2/CO2, which was proven by breakthrough experiments.
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