Abstract
It is imperative to search the eco-friendly and cost-effective technologies for degrading contaminants. Coupling the effect of Ti/PbO2 at the anode with heterogeneous electro-Fenton was an efficient method. Industrial pyrite waste slag characterized by a variety of methods had catalytic performance and stable performance to activate hydrogen peroxide (H2O2) into hydroxyl radical (∙OH). Meanwhile, the processing conditions, the malachite green wastewater concentration, the current density, the pH range, and the dosage of industrial pyrite waste slag were emphatically optimized. Herein, the total organic carbon (TOC) removal efficiency reached 97.70%, the mineralization current efficiency (MCE) was 0.392%, and the energy consumption (EC) was 1.942 kWh/m3 after 240 min. Heterogeneous Ti/PbO2-electro-Fenton using industrial pyrite waste slag as catalyst was an environmentally friendly technology and provided a recycling method with traditional wastes. Finally, catalytic mechanisms and possible pathways were represented according to the results of quantum chemistry calculations and gas chromatography-mass spectrometry (GCMS).
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