Abstract
We report an attractive and efficient synthetic approach to form Si–N bonds via the heterodehydrocoupling of silanes and amines catalyzed by a lanthanum-based N,N-dimethylbenzylamine complex [La(DMBA)3]. A wide variety of primary and secondary amines were well-suited coupling partners with primary, secondary, and tertiary silanes for this catalytic transformation, resulting in the formation of numerous silylamines in high efficiency and moderate-to-excellent yields under mild conditions.
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