Abstract
The conversion of allyl alcohol on SAPO molecular sieves (37, 34, 11 and 5) and H ZSM-5 zeolite at 523–623 K and WHSV=5.1 h −1 results in the formation of diallyl ether, propanal, 2-methyl-2-pentenal and also tetrahydropyran-2-carbaldehyde and 2-oxepanone probably obtained from intermediate acrolein. The catalytic action of the molecular sieves used corresponds to the presence of Brønsted acid sites and basic sites activating the dehydration, dehydrogenation, aldol condensation, Diels–Alder reaction and ring expansion.
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