Abstract

Synthesis of stable main-group element-based radicals represents one of the most interesting topics in contemporary organometallic chemistry because of their vital roles in organic, inorganic, and biological chemistry as well as materials science. However, the access of stable main-group element-based radicals is highly challenging, owing to the lack of energetically accessible orbitals in the main-group elements. In this chapter, we summarize our contribution in the synthesis and characterization of stable heteroatom (N, P, B, S, etc.) centered radical and diradical salts.

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