Abstract
The present understanding of a novel growing class of chain cuprates with intriguing magnetic properties is reviewed. Among them, several undoped edge-shared CuO 2 chain compounds show at low temperature a clear tendency to helicoidal magnetical ordering with acute pitch angles and sometimes also to weak ferromagnetism. Our analysis is based on the isotropic 1D frustrated J 1 – J 2 Heisenberg model with ferromagnetic (FM) 1st neighbor and antiferromagnetic 2nd neighbor exchange. The achieved assignment is supported by microscopic calculations of the electronic and magnetic structure. We consider Na ( Li ) Cu 2 O 2 , LiVCuO 4 as the best studied helimagnets, Li 2 ZrCuO 4 and other systems close to a FM quantum critical point, as well as Li 2 CuO 2 with FM inchain ordering. The interplay of frustrated inchain couplings, anisotropy and interchain exchange is discussed.
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