Abstract
General third-order solutions to the experimental hamiltonian† In this paper the magnetic flux density is denoted by H (as is often the case in chemical applications) rather than by the more correct symbol B. are used to discuss the occurrence, angular dependence and intensities of the ΔMS = 2, ΔMI = 0, ± 1 transitions in transition metal ion systems; both coincident and non-coincident tensor systems are considered. Preliminary results of the ‘half-field’ E.S.R. spectrum of Mn2+ in a natural calcite single crystal is used as an illustration.
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