Abstract
A promising 2.9 µm Ho:GdYTaO4 laser crystal was grown successfully by the Czochralski method for the first time. The crystal belongs to the monoclinic space group of I2/a (No. 15) and high crystalline quality is demonstrated by X-ray rocking curves. The spectral properties of Ho:GdYTaO4 crystal at room temperature are investigated. Based on the Judd–Ofelt theory, the intensity parameters, spontaneous transition probabilities, fluorescence branching ratios, and radiative lifetimes are obtained in detail. The strongest emission peak is located at 2848 nm, and the full width at half maximum is about 15 nm. The experimental lifetimes of 5I6 and 5I7 levels are 0.31 and 8.08 ms, respectively. Moreover, the Stark levels of 5I6, 5I7, and 5I8 are identified and the splitting values are calculated to be 254.1, 226.7, and 370. 4 cm−1, respectively.
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