Abstract
An organic nitronyl nitroxide biradical substituted with a nucleobase of cytosine was designed and synthesized. The molecular ground state of the biradical was found to be triplet (S=1) with a singlet-triplet energy gap of 2J/kB=50.6 K from magnetic susceptibility measurements. The ground-state triplet biradical serves as an S=1 building block for bio-inspired moleculebased magnets with hydrogen-bonded nucleobase pairings.
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