Abstract

We report the ultrashort-pulse Cr:ZnS laser mode-locked by graphene-based saturable absorber mirror. Using the combination of bulk material and a chirped mirror, we demonstrate the shortest reported so far mid-IR pulses of only 5.1 optical cycles (41 fs) centered at 2.4 µm with 190 nm spectral bandwidth. The pulse spectrum almost completely fills the water-free atmospheric window. The output parameters reach 2.3 nJ pulse energy and 250 mW average output power at 108 MHz repetition rate.

Highlights

  • In the recent years, graphene has become a most sought-after saturable absorber for passive mode-locking of lasers

  • The pulse duration of around 50 fs and spectral bandwidth over 120 nm FWHM were reached near the pulse breakup limit

  • The pulse spectrum was centered at 2.37 μm where the calculated intracavity group-delay dispersion is about 400 fs2

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Summary

Introduction

Graphene has become a most sought-after saturable absorber for passive mode-locking of lasers. In practice the absorption may differ from the theoretical value when graphene is doped, or forms bi-, tri- etc. Successful graphene-based femtosecond lasers have been demonstrated for virtually every configuration and in various spectral regions (a recent review can be found in [4], and new results keep arriving almost on a monthly basis). Practical implementations of graphene saturable absorbers (GSA) can take different forms, but for solid-state lasers with sizeable mode diameters, a CVD-based process [5] proved to be quite convenient. A Cr:ZnS laser with this kind of GSA produces up to 250 mW of the shortest to-date generated pulses of 41 fs at 2.4 μm central wavelength

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