Abstract

A new type of broadband saturable absorber made of graphene-Bi2Te3 heterostructure was reported, which synergistically combines light–matter interaction in graphene with that in a small bandgap semiconductor material Bi2Te3 to achieve an improved broadband nonlinear optical response. The graphene-Bi2Te3 heterostructure films were grown by chemical vapor deposition with 15% ${\rm Bi}_{2}{\rm Te}_{3}$ coverage on graphene, in which most of the Bi2Te3 nanoplatelets are less than 30 nm thick. It is interesting to find that the heterostructure thin film shows broadband saturable absorption property. At the communication band (around 1560 nm), the saturable intensity and modulation depth are measured to be 4.95 MW/cm2 and 18.98%, respectively. While around 1067 nm, the corresponding saturable intensity and modulation depth are experimentally measured to be 2.61 MW/cm2 and 23.11%, respectively. By incorporating this optical saturable absorber inside either an Er-doped or Yb-doped fiber laser, we are able to generate ultra-short pulse with very stable operation at 1565.6 and 1049.1 nm. Our experimental results clearly demonstrate that the graphene-Bi 2Te3 heterostructure can be a promising broadband nonlinear optical material for broadband ultra-fast laser photonics.

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