Abstract

The formation of a gradient of atomic oxygen is demonstrated by means of a nanosecond non-equilibrium plasma for a varying gap size plane-to-plane electrode. Using a flat high-voltage electrode in front of a rounded triangle a 2.9 to 5 cm gap is formed over a 9.8 cm span. ICCD imaging determined an adequate ground electrode shape and slope to create a gradient. The plasma is formed by three consecutive high voltage pulses of -30, -40 and -50 kV in 100 mbar of air. O-TALIF measurements confirm that atomic oxygen production changed with gap size within the same plasma. This setup will be used to test detonation initiation by Zel’dovich gradient mechanisms in stoichiometric H2:O2 mixtures.Novelty and Significance: A novel configuration of a nanosecond non-equilibrium discharge was developed to create a controllable gradient of atomic oxygen. This was achieved by using varying gap plane-to-plane electrodes to generate an electric field of varying strength along the length of the gap. This setup will be tested in combustible mixtures to initiate a detonation wave using a gradient mechanism of Zel’dovich.

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