Glass quantization of the Gaussian core model.

Abstract

We use the replica method to study the dynamical glass transition of the Gaussian core model, a system of ultrasoft repulsive spheres interacting via a Gaussian potential, focusing on low temperatures and low-to-moderate densities. At constant temperature, an amorphous glassy state is entered upon a first compression but this glass melts as the density is further increased. In addition to this reentrant transition, a second, smooth transition is discovered between a continuous and a discretized glass. The properties of the former are continuous functions of temperatures, whereas the latter exhibits a succession of stripes, characterized by discontinuous jumps of the glassiness parameters. The glass physics of ultrasoft particles is hence richer than that of impenetrable particles for reasons that can be attributed to the ability of the former to create and break out-of-equilibrium clusters of overlapping particles.