Abstract
SynopsisGeometrical reconstructions are performed for Carbonyl Sulfide (OCS) through Coulomb Explosion Imaging (CEI) employing intense femtosecond laser ionization with pulse durations 7 fs, 30 fs, 60 fs, 100 fs, and 200 fs, using two methods that significantly differ in approach. Firstly, a look up table is employed to reconstruct OCS (2, 2, 2) channel and highlight the presence of degenerate regions. Following this a more sophisticated constrained nonlinear optimization approach improves on precision and gives an indication of uncertainty. Results are compared with equilibrium geometry.
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