Abstract
Fourth-harmonic pulses of a 1 kHz chirped-pulse amplification (CPA) Ti:sapphire laser have been generated by a scheme of dual broadband frequency doubling with two β-BaB2O4 (BBO) crystals. The pulse energy was 90 µJ with a bandwidth of 2.7 nm (full width at half maximum, FWHM) at a central wavelength of 220 nm. The pulse width was measured to be 45 fs by autocorrelation with the two-photon fluorescence of CaF2, which was much smaller than that (120 fs) obtained by conventional frequency conversion.
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