Abstract

Phase-stable half-cycle mid-infrared pulses were produced through filamentation in argon. The pulse width was obtained as 7.9 fs at 4.1 μm carrier wave length by using frequency-resolved optical gating.

Highlights

  • Filamentation of powerful ultrashort laser pulses in gases [1,2,3] is one of the most interesting phenomena in nonlinear optics

  • Such MIR pulses with more than one octave at full width at half maximum are very attractive to be applied for molecular spectroscopy, e.g. two-dimensional infrared spectroscopy

  • We report the latest progress of the ultrabroadband MIR pulse generation through filamentation

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Summary

Introduction

Filamentation of powerful ultrashort laser pulses in gases [1,2,3] is one of the most interesting phenomena in nonlinear optics. Enhanced nonlinear-optical processes in laser-induced filaments suggest a new strategy for the generation of ultrashort pulses of long-wavelength radiation. Ultrabroadband mid-infrared (MIR, 3– 20 μm) pulse generation through filamentation in air was firstly demonstrated in 2007 [4], and the technique was followed by several groups [5,6,7].

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