Abstract
Instead of the 1,2-alkyl migration well-established for carbocyclic analogues, the 1,3-radical cation 1˙+, generated from the corresponding housane 1 by oxidation with (4-BrC6H4)3N˙+SbCl, undergoes an unexpected deprotonation to give the monoradical (1H)˙. In this process the proton is presumably transferred to one of the two carbonyl groups of the triazolidinedione ring.
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