Abstract
Time resolved spectroscopic investigations of ultrafast processes at surfaces or in gaseous media, e. g. photodissociation and fragmentation of molecules and clusters 1,2 require femtosecond pulses tunable in the vacuum ultraviolet (VUV) spectral range. Clusters show for instance a very strong dependence of the absorption peak on the their size. The region between 100nm-150nm is of special interest for small clusters. Single photon ionization will be possible for photons of this energy range.
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