Abstract

We propose a systematic and sequential expansion of the Landau–Lifshitz–Gilbert equation utilizing the dependence of the Gilbert damping tensor on the angle between magnetic moments, which arises from multi-body scattering processes. The tensor consists of a damping-like term and a correction to the gyromagnetic ratio. Based on electronic structure theory, both terms are shown to depend on e.g. the scalar, anisotropic, vector-chiral and scalar-chiral products of magnetic moments: e i ⋅ e j , (n ij ⋅ e i )(n ij ⋅ e j ), n ij ⋅ (e i × e j ), , e i ⋅ (e j × e k ) …, where some terms are subjected to the spin–orbit field n ij in first and second order. We explore the magnitude of the different contributions using both the Alexander–Anderson model and time-dependent density functional theory in magnetic adatoms and dimers deposited on Au(111) surface.

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