Gas-liquid mass transfer in a gas–liquid-solid three-phase moving bed

Abstract

The gas–liquid mass transfer was investigated in a gas–liquid-solid three-phase moving bed based on the dissolved oxygen method, and a semi-quantitative gas–liquid boundary identification method was developed to measure the gas–liquid interfacial area. Results showed that the effects of gas velocity and liquid velocity on gas–liquid mass transfer in the three-phase moving bed were the same as those in the trickle bed. Since the gas–liquid interfacial area and its renewal speed were promoted at the low particle velocity and inhibited at the high particle velocity, the liquid-phase volumetric mass-transfer coefficient first increased and then decreased with the increasing particle velocity. Moreover, an empirical correlation for the liquid-phase volumetric mass-transfer coefficient was established based on 296 data, and the average relative deviation was 8.11%. The sensitivity analysis showed that the liquid velocity was more important to gas–liquid mass transfer than gas velocity and particle velocity.