Abstract

Free-molecule perpendicular g factor shifts (Δ g⊥) of the CN and C 2H radicals, determined by analysis of high resolution ESR spectra of the radicals in Ar and Kr matrices at 4K, support the predicted relation γ = 2 B OΔ g⊥, where γ and B O are the spin doubling and rotational constants. The analysis also shows that CN in Ar at 4 K undergoes a complex motion resulting in a nonaxial spin hamiltonian.

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