Abstract

Abstract The coexistence of seemingly mutually exclusive properties such as ferromagnetism, ferroelectricity and metallicity in atomically thin materials is the requirement of the hour in electronics as the Moore’s law faces an impending end. Only a few 2D multiferroic materials have been predicted/realized so far. The polar metals with simultaneous presence of polarity and conductivity are also equally rare. Here, we predict, based on first-principles calculations that an Eu-substituted rare-earth halide GdI2 monolayer showcases ferromagnetism, ferroelasticity while being polar and a fully spin-polarized semi-metal at the same time. The ferroelasticity and polarity are shown to be coupled making it possible to switch the polar direction using external mechanical stress. Further, it is observed that an application of biaxial tensile strain of 5% causes the spin easy-axis to shift from out-of-plane to in-plane direction. Thus, spin easy axis gets coupled with the direction of polarization in the strained monolayer making the switching of magnetization also possible using external strain. Simultaneous coexistence and coupling of the ferroic orders in a metallic 2D material makes the Eu substituted GdI2 monolayer an incredibly rare material for nano-electronics and spintronics applications.

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