Abstract
The symmetry principles governing the non-linear interaction of intense laser radiation with molecular ensembles show that dynamical interaction phenomena exist in the ensemble even though the induced frequency dependent polarisation be purely imaginary, and unobservable in the static limit. An example is computer simulated in the S enantiomer of bromochlorofluoromethane, showing clear effects on the orientational and rotational velocity correlation functions and by Fourier transform, the dielectric and far infra red spectra. Conditions are suggested for its experimental observation and order of magnitudies calculated for the appropriate mediating tensors.
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