Abstract

Quantum spin liquids (QSLs) are exotic states of matter characterized by emergent gauge structures and fractionalized elementary excitations. The recently discovered triangular lattice antiferromagnet YbMgGaO4 is a promising QSL candidate, and the nature of its ground state is still under debate. Here we use neutron scattering to study the spin excitations in YbMgGaO4 under various magnetic fields. Our data reveal a dispersive spin excitation continuum with clear upper and lower excitation edges under a weak magnetic field (H = 2.5 T). Moreover, a spectral crossing emerges at the Γ point at the Zeeman-split energy. The corresponding redistribution of the spectral weight and its field-dependent evolution are consistent with the theoretical prediction based on the inter-band and intra-band spinon particle-hole excitations associated with the Zeeman-split spinon bands, implying the presence of fractionalized excitations and spinon Fermi surfaces in the partially magnetized QSL state in YbMgGaO4.

Highlights

  • Quantum spin liquids (QSLs) are exotic states of matter characterized by emergent gauge structures and fractionalized elementary excitations

  • In a weak magnetic field of H = 2.5 T applied along the c-axis, a dispersive spin excitation continuum is revealed with clear upper and lower excitations edges, leading to a spectral crossing at the Γ point at the Zeeman-split energy

  • We propose that the modulation of the spectral weights of the continuum in the low-field regime is consistent with the previously predicted behavior of the spinon Fermi surface QSL state under magnetic fields[30]

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Summary

Introduction

Quantum spin liquids (QSLs) are exotic states of matter characterized by emergent gauge structures and fractionalized elementary excitations. The corresponding redistribution of the spectral weight and its field-dependent evolution are consistent with the theoretical prediction based on the inter-band and intra-band spinon particle-hole excitations associated with the Zeeman-split spinon bands, implying the presence of fractionalized excitations and spinon Fermi surfaces in the partially magnetized QSL state in YbMgGaO4. For the spin-1/2 Heisenberg chain, which is essentially a one-dimensional Luttinger liquid, and is not a true QSL in the modern sense, but shows spinon excitations in the form of domain walls, the external magnetic field could lead to the splitting of the spinon band, resulting in a modulation and redistribution of the spinon continuum[32,33] These results provided a firm confirmation of the fractionalized spinon excitation in one spatial dimension. Our results provide an important piece of evidence for fractionalized spinon excitations and spinon Fermi surfaces in YbMgGaO4 under magnetic fields

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