Abstract
The rotational spectra of CoNO were measured using a Fourier-transform microwave (FTMW) spectrometer. The CoNO molecules were generated in supersonic jets using the pulse-discharge reaction of Co(CO)3NO diluted with Ar. The amount of CoNO generated under the present experimental conditions was significantly more than that of CoCO, although the CO contained in a molecule of the precursor Co(CO)3NO is three times more than NO. The quadrupole parameter of the N nucleus was determined for a transition metal mononitrosyl complex for the first time and compared with those of other nitrosyl compounds.
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